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Demand for high-capacity data exchange, precise quality monitoring, and detection of environmentally or health-relevant agents is nowadays a main drive of scientific innovation. Quantum effects at the single-particle level offers the potential for exponentially faster computing, secure communications, and unparalleled sensing through the implementation of the so-called “quantum technologies”.

Single polyaromatic hydrocarbon (PAH) molecules in suitable hosts exhibit coherent light interactions at low temperatures. When efficiently coupled to nanophotonic devices, these molecules can act as both single-photon sources and nonlinear elements, enabling on-chip single-photon quantum logic gates.

Our research focuses on devices combining Dibenzoterrylene (DBT) molecules in anthracene crystals with dielectric waveguides and other various photonic structures. These emitters feature exceptional photostability, strong dipole transitions in the near-infrared (780 nm), and lifetime-limited linewidths of 30 MHz at 3 K. We are exploring various photonic designs, including materials like Si3N4 and polymers, and investigating both theoretical and experimental approaches.

A schematic illustration of the main features of organic molecules as single photon sources. The HOMO-LUMO transition behaves like an atomic transition, emitting a single photon per time, as visible from the photon statistics. These molecular sources based on polycyclic aromatic hydrocarbons are bright and stable, exhibiting exceptional coherence properties.
In this GIF we see a large sublimated antracene crystal doped with DBT molecules under continuous wave excitation. The total sample size is on the tens of micrometers size, while the bright spots are isolated molecules that are brought in and out of resonance.

Selected publications

Real-time two-photon interference from distinct molecules on the same chip

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Enhanced control of single-molecule emission frequency and spectral diffusion

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Advances in Quantum Metrology with Dielectrically Structured Single Photon Sources Based on Molecules

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Laser-Induced Frequency Tuning of Fourier-Limited Single-Molecule Emitters

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Self-Assembled Nanocrystals of Polycyclic Aromatic Hydrocarbons Show Photostable Single-Photon Emission

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A 3D Polymeric Platform for Photonic Quantum Technologies

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Photostable molecules on chip: integrated single photon sources for quantum technologies

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A realistic fabrication and design concept for quantum gates based on single emitters integrated in plasmonic-dielectric waveguide structures

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Single organic molecules for photonic quantum technologies

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A Molecule-Based Single-Photon Source Applied in Quantum Radiometry

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Triggered emission of indistinguishable photons from an organic dye molecule

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Beaming light from a quantum emitter with a planar optical antenna

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Efficient room-temperature molecular single-photon sources for quantum key distribution

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